Synthetic Geopolymers for Controlled Delivery of Oxycodone: Adjustable and Nanostructured Porosity Enables Tunable and Sustained Drug Release
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{"title"=>"Synthetic geopolymers for controlled delivery of oxycodone: Adjustable and nanostructured porosity enables tunable and sustained drug release", "type"=>"journal", "authors"=>[{"first_name"=>"Johan", "last_name"=>"Forsgren", "scopus_author_id"=>"21733254000"}, {"first_name"=>"Christian", "last_name"=>"Pedersen", "scopus_author_id"=>"57198011378"}, {"first_name"=>"Maria", "last_name"=>"Strømme", "scopus_author_id"=>"56249828500"}, {"first_name"=>"Håkan", "last_name"=>"Engqvist", "scopus_author_id"=>"56243269100"}], "year"=>2011, "source"=>"PLoS ONE", "identifiers"=>{"sgr"=>"79952649512", "pui"=>"361447252", "doi"=>"10.1371/journal.pone.0017759", "pmid"=>"21423616", "scopus"=>"2-s2.0-79952649512", "issn"=>"19326203", "isbn"=>"1932-6203"}, "id"=>"ae5d8f35-af53-32ee-b660-0e032867b331", "abstract"=>"In this article we for the first time present a fully synthetic mesoporous geopolymer drug carrier for controlled release of opioids. Nanoparticulate precursor powders with different Al/Si-ratios were synthesized by a sol-gel route and used in the preparation of different geopolymers, which could be structurally tailored by adjusting the Al/Si-ratio and the curing temperatures. In particular, it was shown that the pore sizes of the geopolymers decreased with increasing Al/Si ratio and that completely mesoporous geopolymers could be produced from precursor particles with the Al/Si ratio 2:1. The mesoporosity was shown to be associated with a sustained and linear in vitro release profile of the opioid oxycodone. A clinically relevant release period of about 12 h was obtained by adjusting the size of the pellets. The easily fabricated and tunable geopolymers presented in this study constitute a novel approach in the development of controlled release formulations, not only for opioids, but whenever the clinical indication is best treated with a constant supply of drugs and when the mechanical stability of the delivery vehicle is crucial.", "link"=>"http://www.mendeley.com/research/synthetic-geopolymers-controlled-delivery-oxycodone-adjustable-nanostructured-porosity-enables-tunab", "reader_count"=>29, "reader_count_by_academic_status"=>{"Unspecified"=>1, "Professor > Associate Professor"=>2, "Researcher"=>8, "Student > Doctoral Student"=>2, "Student > Ph. D. Student"=>8, "Student > Postgraduate"=>1, "Student > Master"=>3, "Student > Bachelor"=>3, "Professor"=>1}, "reader_count_by_user_role"=>{"Unspecified"=>1, "Professor > Associate Professor"=>2, "Researcher"=>8, "Student > Doctoral Student"=>2, "Student > Ph. D. Student"=>8, "Student > Postgraduate"=>1, "Student > Master"=>3, "Student > Bachelor"=>3, "Professor"=>1}, "reader_count_by_subject_area"=>{"Engineering"=>6, "Unspecified"=>3, "Biochemistry, Genetics and Molecular Biology"=>1, "Materials Science"=>6, "Agricultural and Biological Sciences"=>3, "Medicine and Dentistry"=>1, "Pharmacology, Toxicology and Pharmaceutical Science"=>1, "Business, Management and Accounting"=>1, "Physics and Astronomy"=>1, "Chemistry"=>6}, "reader_count_by_subdiscipline"=>{"Engineering"=>{"Engineering"=>6}, "Materials Science"=>{"Materials Science"=>6}, "Medicine and Dentistry"=>{"Medicine and Dentistry"=>1}, "Chemistry"=>{"Chemistry"=>6}, "Physics and Astronomy"=>{"Physics and Astronomy"=>1}, "Agricultural and Biological Sciences"=>{"Agricultural and Biological Sciences"=>3}, "Business, Management and Accounting"=>{"Business, Management and Accounting"=>1}, "Biochemistry, Genetics and Molecular Biology"=>{"Biochemistry, Genetics and Molecular Biology"=>1}, "Unspecified"=>{"Unspecified"=>3}, "Pharmacology, Toxicology and Pharmaceutical Science"=>{"Pharmacology, Toxicology and Pharmaceutical Science"=>1}}, "reader_count_by_country"=>{"Argentina"=>1, "Cameroon"=>1, "Turkey"=>1, "Poland"=>1}, "group_count"=>2}

Scopus | Further Information

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Figshare

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  • {"files"=>["https://ndownloader.figshare.com/files/791634"], "description"=>"<p>Names and synthesis conditions of drug containing geopolymer samples.</p>", "links"=>[], "tags"=>["synthesis", "conditions", "containing", "geopolymer"], "article_id"=>462004, "categories"=>["Chemistry"], "users"=>["Johan Forsgren", "Christian Pedersen", "Maria Strømme", "Håkan Engqvist"], "doi"=>"https://dx.doi.org/10.1371/journal.pone.0017759.t003", "stats"=>{"downloads"=>0, "page_views"=>7, "likes"=>0}, "figshare_url"=>"https://figshare.com/articles/_Names_and_synthesis_conditions_of_drug_containing_geopolymer_samples_/462004", "title"=>"Names and synthesis conditions of drug containing geopolymer samples.", "pos_in_sequence"=>0, "defined_type"=>3, "published_date"=>"2013-02-20 19:55:57"}
  • {"files"=>["https://ndownloader.figshare.com/files/791338"], "description"=>"<p>Pore size distributions in the geopolymer samples.</p>", "links"=>[], "tags"=>["distributions", "geopolymer"], "article_id"=>461710, "categories"=>["Chemistry"], "users"=>["Johan Forsgren", "Christian Pedersen", "Maria Strømme", "Håkan Engqvist"], "doi"=>"https://dx.doi.org/10.1371/journal.pone.0017759.g004", "stats"=>{"downloads"=>0, "page_views"=>8, "likes"=>0}, "figshare_url"=>"https://figshare.com/articles/_Pore_size_distributions_in_the_geopolymer_samples_/461710", "title"=>"Pore size distributions in the geopolymer samples.", "pos_in_sequence"=>0, "defined_type"=>1, "published_date"=>"2013-02-20 19:54:22"}
  • {"files"=>["https://ndownloader.figshare.com/files/791558"], "description"=>"<p>Comparison of release profiles for DR21-60 in pH 6.8 and in 40% ethanol, and for DR11-60 in pH 6.8 and pH 1.0 (pellet dimensions Ø: 1.5 mm · h: 1.5 mm).</p>", "links"=>[], "tags"=>["profiles", "ph", "40"], "article_id"=>461931, "categories"=>["Chemistry"], "users"=>["Johan Forsgren", "Christian Pedersen", "Maria Strømme", "Håkan Engqvist"], "doi"=>"https://dx.doi.org/10.1371/journal.pone.0017759.g008", "stats"=>{"downloads"=>0, "page_views"=>2, "likes"=>0}, "figshare_url"=>"https://figshare.com/articles/_Release_profiles_in_pH_6_8_and_in_40_vol_ethanol_/461931", "title"=>"Release profiles in pH 6.8 and in 40 vol% ethanol.", "pos_in_sequence"=>0, "defined_type"=>1, "published_date"=>"2013-02-20 19:55:34"}
  • {"files"=>["https://ndownloader.figshare.com/files/791095"], "description"=>"<p>1) First, precursor powders are made in a sol-gel process. 2) Thereafter, the powder is mixed with a sodium silicate solution to form a paste that is transferred to moulds and left to cure. For drug release experiments oxycodone HCL is added to the paste before moulding. 3) After curing the pellets are removed from the mould. The particular pellets in panel 3 have the dimensions Ø: 1.5 mm · h: 1.5 mm and contains oxycodone.</p>", "links"=>[], "tags"=>["pellet"], "article_id"=>461468, "categories"=>["Chemistry"], "users"=>["Johan Forsgren", "Christian Pedersen", "Maria Strømme", "Håkan Engqvist"], "doi"=>"https://dx.doi.org/10.1371/journal.pone.0017759.g001", "stats"=>{"downloads"=>1, "page_views"=>4, "likes"=>0}, "figshare_url"=>"https://figshare.com/articles/_Geopolymer_pellet_synthesis_/461468", "title"=>"Geopolymer pellet synthesis.", "pos_in_sequence"=>0, "defined_type"=>1, "published_date"=>"2013-02-20 19:52:55"}
  • {"files"=>["https://ndownloader.figshare.com/files/791286"], "description"=>"<p>N<sub>2</sub> isotherms for the geopolymer samples.</p>", "links"=>[], "tags"=>["isotherms", "geopolymer"], "article_id"=>461657, "categories"=>["Chemistry"], "users"=>["Johan Forsgren", "Christian Pedersen", "Maria Strømme", "Håkan Engqvist"], "doi"=>"https://dx.doi.org/10.1371/journal.pone.0017759.g003", "stats"=>{"downloads"=>2, "page_views"=>18, "likes"=>0}, "figshare_url"=>"https://figshare.com/articles/_N_2_isotherms_for_the_geopolymer_samples_/461657", "title"=>"N<sub>2</sub> isotherms for the geopolymer samples.", "pos_in_sequence"=>0, "defined_type"=>1, "published_date"=>"2013-02-20 19:54:04"}
  • {"files"=>["https://ndownloader.figshare.com/files/791504"], "description"=>"<p>Oxycodone is released in pH 6.8, from DR11-RT pellets of two different dimensions: (i) Ø: 0.5 mm · h: 1.0 mm and (ii) Ø: 1.5 mm · h: 1.5 mm</p>", "links"=>[], "tags"=>["pellet"], "article_id"=>461880, "categories"=>["Chemistry"], "users"=>["Johan Forsgren", "Christian Pedersen", "Maria Strømme", "Håkan Engqvist"], "doi"=>"https://dx.doi.org/10.1371/journal.pone.0017759.g007", "stats"=>{"downloads"=>0, "page_views"=>4, "likes"=>0}, "figshare_url"=>"https://figshare.com/articles/_Influence_of_pellet_size_on_drug_release_profile_/461880", "title"=>"Influence of pellet size on drug release profile.", "pos_in_sequence"=>0, "defined_type"=>1, "published_date"=>"2013-02-20 19:55:19"}
  • {"files"=>["https://ndownloader.figshare.com/files/791442"], "description"=>"<p>Each curve show the total release of oxycodone from roughly 135 pellets (weighing in total 600 mg) with the dimensions Ø: 1.5 mm · h: 1.5 mm.</p>", "links"=>[], "tags"=>["profiles", "ph", "oxycodone", "carrying", "geopolymer"], "article_id"=>461811, "categories"=>["Chemistry"], "users"=>["Johan Forsgren", "Christian Pedersen", "Maria Strømme", "Håkan Engqvist"], "doi"=>"https://dx.doi.org/10.1371/journal.pone.0017759.g006", "stats"=>{"downloads"=>1, "page_views"=>5, "likes"=>0}, "figshare_url"=>"https://figshare.com/articles/_Release_profiles_in_pH_6_8_for_the_oxycodone_carrying_geopolymer_samples_/461811", "title"=>"Release profiles in pH 6.8 for the oxycodone carrying geopolymer samples.", "pos_in_sequence"=>0, "defined_type"=>1, "published_date"=>"2013-02-20 19:54:57"}
  • {"files"=>["https://ndownloader.figshare.com/files/791659"], "description"=>"<p>The name of each geopolymer sample refers to the Al/Si molar ratio of its precursor powder.</p>", "links"=>[], "tags"=>["geopolymer"], "article_id"=>462034, "categories"=>["Chemistry"], "users"=>["Johan Forsgren", "Christian Pedersen", "Maria Strømme", "Håkan Engqvist"], "doi"=>"https://dx.doi.org/10.1371/journal.pone.0017759.t002", "stats"=>{"downloads"=>1, "page_views"=>6, "likes"=>0}, "figshare_url"=>"https://figshare.com/articles/_Characteristics_of_geopolymer_samples_/462034", "title"=>"Characteristics of geopolymer samples.", "pos_in_sequence"=>0, "defined_type"=>3, "published_date"=>"2013-02-20 19:56:07"}

PMC Usage Stats | Further Information

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Relative Metric

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