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Predictive models of poly(ethylene-terephthalate) film degradation under multi-factor accelerated weathering exposures

Publication Date: May 12, 2017
Authors: Abdulkerim Gok, David K. Ngendahimana, Cara L. Fagerholm, Roger H. French, et al
Volume: 12
Issue: 5
Pages: e0177614
DOI: https://dx.plos.org/10.1371/journal.pone.0177614
Publisher URL: http://journals.plos.org/plosone/article?id=10.1371%2Fjournal.pone.0177614
Scopus: 85019461166
Mendeley: http://www.mendeley.com/research/predictive-models-polyethyleneterephthalate-film-degradation-under-multifactor-accelerated-weatherin

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Mendeley 1111 May 15:11 UTC

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{"title"=>"Predictive models of poly(ethyleneterephthalate) film degradation under multifactor accelerated weathering exposures", "type"=>"journal", "authors"=>[{"first_name"=>"Abdulkerim", "last_name"=>"Gok", "scopus_author_id"=>"56513620000"}, {"first_name"=>"David K.", "last_name"=>"Ngendahimana", "scopus_author_id"=>"57194233656"}, {"first_name"=>"Cara L.", "last_name"=>"Fagerholm", "scopus_author_id"=>"57015452600"}, {"first_name"=>"Roger H.", "last_name"=>"French", "scopus_author_id"=>"7202789368"}, {"first_name"=>"Jiayang", "last_name"=>"Sun", "scopus_author_id"=>"7410369151"}, {"first_name"=>"Laura S.", "last_name"=>"Bruckman", "scopus_author_id"=>"55453912900"}], "year"=>2017, "source"=>"PLoS ONE", "identifiers"=>{"issn"=>"19326203", "scopus"=>"2-s2.0-85019461166", "sgr"=>"85019461166", "pui"=>"616160590", "isbn"=>"1111111111", "doi"=>"10.1371/journal.pone.0177614"}, "id"=>"161b02e7-9658-3e5f-a00e-30f61586719f", "abstract"=>"© 2017 Gok et al. This is an open access article distributed under the terms of the Creative Commons Attribution License, which permits unrestricted use, distribution, and reproduction in any medium, provided the original author and source are credited.Accelerated weathering exposures were performed on poly(ethylene-terephthalate) (PET) films. Longitudinal multi-level predictive models as a function of PET grades and exposure types were developed for the change in yellowness index (YI) and haze (%). Exposures with similar change in YI were modeled using a linear fixed-effects modeling approach. Due to the complex nature of haze formation, measurement uncertainty, and the differences in the samples' responses, the change in haze (%) depended on individual samples' responses and a linear mixed-effects modeling approach was used. When compared to fixed-effects models, the addition of random effects in the haze formation models significantly increased the variance explained. For both modeling approaches, diagnostic plots confirmed independence and homogeneity with normally distributed residual errors. Predictive R2 values for true prediction error and predictive power of the models demonstrated that the models were not subject to over-fitting. These models enable prediction under pre-defined exposure conditions for a given exposure time (or photo-dosage in case of UV light exposure). PET degradation under cyclic exposures combining UV light and condensing humidity is caused by photolytic and hydrolytic mechanisms causing yellowing and haze formation. Quantitative knowledge of these degradation pathways enable cross-correlation of these lab-based exposures with real-world conditions for service life prediction.", "link"=>"http://www.mendeley.com/research/predictive-models-polyethyleneterephthalate-film-degradation-under-multifactor-accelerated-weatherin", "reader_count"=>11, "reader_count_by_academic_status"=>{"Unspecified"=>2, "Researcher"=>3, "Student > Ph. D. Student"=>2, "Student > Master"=>2, "Student > Bachelor"=>1, "Professor"=>1}, "reader_count_by_user_role"=>{"Unspecified"=>2, "Researcher"=>3, "Student > Ph. D. Student"=>2, "Student > Master"=>2, "Student > Bachelor"=>1, "Professor"=>1}, "reader_count_by_subject_area"=>{"Engineering"=>3, "Unspecified"=>2, "Biochemistry, Genetics and Molecular Biology"=>2, "Materials Science"=>3, "Energy"=>1}, "reader_count_by_subdiscipline"=>{"Engineering"=>{"Engineering"=>3}, "Materials Science"=>{"Materials Science"=>3}, "Energy"=>{"Energy"=>1}, "Biochemistry, Genetics and Molecular Biology"=>{"Biochemistry, Genetics and Molecular Biology"=>2}, "Unspecified"=>{"Unspecified"=>2}}, "group_count"=>0}

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Web of Science®14 Apr 06:31 UTC

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